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Lawrence Que

This is a preview profile on BiomedExperts - the first literature-based scientific social network. It brings the right researchers together and allows them to collaborate online. Collexis and Dell provide the BiomedExperts network of +1.5 Million pre-calculated profiles free of charge to researchers worldwide.

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Co-Publications
Name
29
Münck, Eckard
23
Costas, Miquel
18
Rohde, Jan-Uwe
14
Stubna, Audria
13
Nam, Wonwoo
13
Ho, Raymond
11
Bukowski, Michael
10
Bominaar, Emile
10
Lipscomb, John
10
Rybak-Akimova, Elena
10
Shan, Xiaopeng
9
Mehn, Mark
9
Solomon, Edward
9
Mas-Ballesté, Rubén
9
Kaizer, József

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Publications

TOP 3
Vu Van V; Emerson Joseph P; Martinho Marlène; Kim Yeon Sook; Münck Eckard; Park Myung Hee; Que Lawrence
Human deoxyhypusine hydroxylase, an enzyme involved in regulating cell growth, activates O2 with a nonheme diiron center.
Frisch Jonathan R; Vu Van V; Martinho Marlène; Münck Eckard; Que Lawrence
Characterization of two distinct adducts in the reaction of a nonheme diiron(II) complex with O2.
Martinho Marlène; Xue Genqiang; Fiedler Adam T; Que Lawrence; Bominaar Emile L; Münck Eckard
Mössbauer and DFT study of the ferromagnetically coupled diiron(IV) precursor to a complex with an Fe(IV)(2)O(2) diamond core.

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All Publications

2009: Vu Van V; Emerson Joseph P; Martinho Marlène; Kim Yeon Sook; Münck Eckard; Park Myung Hee; Que Lawrence
Human deoxyhypusine hydroxylase, an enzyme involved in regulating cell growth, activates O2 with a nonheme diiron center.
Proceedings of the National Academy of Sciences of the United States of America 2009;106(35):14814-9.
2009: Frisch Jonathan R; Vu Van V; Martinho Marlène; Münck Eckard; Que Lawrence
Characterization of two distinct adducts in the reaction of a nonheme diiron(II) complex with O2.
Inorganic chemistry 2009;48(17):8325-36.
2009: Martinho Marlène; Xue Genqiang; Fiedler Adam T; Que Lawrence; Bominaar Emile L; Münck Eckard
Mössbauer and DFT study of the ferromagnetically coupled diiron(IV) precursor to a complex with an Fe(IV)(2)O(2) diamond core.
Journal of the American Chemical Society 2009;131(16):5823-30.
2009: England Jason; Martinho Marlène; Farquhar Erik R; Frisch Jonathan R; Bominaar Emile L; Münck Eckard; Que Lawrence
A synthetic high-spin oxoiron(IV) complex: generation, spectroscopic characterization, and reactivity.
Angewandte Chemie (International ed. in English) 2009;48(20):3622-6.
2009: Company Anna; Feng Yan; Güell Mireia; Ribas Xavi; Luis Josep M; Que Lawrence; Costas Miquel
Olefin-dependent discrimination between two nonheme HO-FeV=O tautomeric species in catalytic H2O2 epoxidations.
Chemistry (Weinheim an der Bergstrasse, Germany) 2009;15(14):3359-62.
2009: Mukherjee Anusree; Martinho Marlène; Bominaar Emile L; Münck Eckard; Que Lawrence
Shape-selective interception by hydrocarbons of the O2-derived oxidant of a biomimetic nonheme iron complex.
Angewandte Chemie (International ed. in English) 2009;48(10):1780-3.
2009: Klinker Eric J; Shaik Sason; Hirao Hajime; Que Lawrence
A two-state reactivity model explains unusual kinetic isotope effect patterns in C-H bond cleavage by nonheme oxoiron(IV) complexes.
Angewandte Chemie (International ed. in English) 2009;48(7):1291-5.
2008: Fiedler Adam T; Shan Xiaopeng; Mehn Mark P; Kaizer József; Torelli Stéphane; Frisch Jonathan R; Kodera Masahito; Que Lawrence
Spectroscopic and computational studies of (mu-oxo)(mu-1,2-peroxo)diiron(III) complexes of relevance to nonheme diiron oxygenase intermediates.
The journal of physical chemistry. A 2008;112(50):13037-44.
2008: Que Lawrence; Tolman William B
Biologically inspired oxidation catalysis.
Nature 2008;455(7211):333-40.
2008: Jackson Timothy A; Rohde Jan-Uwe; Seo Mi Sook; Sastri Chivukula V; DeHont Raymond; Stubna Audria; Ohta Takehiro; Kitagawa Teizo; Münck Eckard; Nam Wonwoo; Que Lawrence
Axial ligand effects on the geometric and electronic structures of nonheme oxoiron(IV) complexes.
Journal of the American Chemical Society 2008;130(37):12394-407.
2008: Emerson Joseph P; Kovaleva Elena G; Farquhar Erik R; Lipscomb John D; Que Lawrence
Swapping metals in Fe- and Mn-dependent dioxygenases: evidence for oxygen activation without a change in metal redox state.
Proceedings of the National Academy of Sciences of the United States of America 2008;105(21):7347-52.
2008: Shan Xiaopeng; Que Lawrence
Unexpected kinetic complexity in the formation of a nonheme oxoiron(IV) complex.
Chemical communications (Cambridge, England) 2008;(19):2209-11.
2008: Chanda Arani; Shan Xiaopeng; Chakrabarti Mrinmoy; Ellis W Chadwick; Popescu Delia L; Tiago de Oliveira Filipe; Wang Dong; Que Lawrence; Collins Terrence J; Münck Eckard; Bominaar Emile L
(TAML)FeIV O complex in aqueous solution: synthesis and spectroscopic and computational characterization.
Inorganic chemistry 2008;47(9):3669-78.
2008: Mas-Balleste Ruben; Fujita Megumi; Que Lawrence
High-valent iron-mediated cis-hydroxyacetoxylation of olefins.
Dalton transactions (Cambridge, England : 2003) 2008;(14):1828-30.
2008: Bell Caleb B; Wong Shaun D; Xiao Yuming; Klinker Eric J; Tenderholt Adam L; Smith Matt C; Rohde Jan-Uwe; Que Lawrence; Cramer Stephen P; Solomon Edward I
A combined NRVS and DFT study of Fe(IV)=O model complexes: a diagnostic method for the elucidation of non-heme iron enzyme intermediates.
Angewandte Chemie (International ed. in English) 2008;47(47):9071-4.
2008: Ray Kallol; England Jason; Fiedler Adam T; Martinho Marlène; Münck Eckard; Que Lawrence
An inverted and more oxidizing isomer of [Fe(IV)(O)(tmc)(NCCH3)]2+.
Angewandte Chemie (International ed. in English) 2008;47(42):8068-71.
2008: Company Anna; Palavicini Sara; Garcia-Bosch Isaac; Mas-Ballesté Ruben; Que Lawrence; Rybak-Akimova Elena V; Casella Luigi; Ribas Xavi; Costas Miquel
Tyrosinase-like reactivity in a Cu(III)2(mu-O)2 species.
Chemistry (Weinheim an der Bergstrasse, Germany) 2008;14(12):3535-8.
2008: Zhou Yuming; Shan Xiaopeng; Mas-Ballesté Rubén; Bukowski Michael R; Stubna Audria; Chakrabarti Mrinmoy; Slominski Luke; Halfen Jason A; Münck Eckard; Que Lawrence
Contrasting cis and trans effects on the reactivity of nonheme oxoiron(IV) complexes.
Angewandte Chemie (International ed. in English) 2008;47(10):1896-9.
2007: Xue Genqiang; Wang Dong; De Hont Raymond; Fiedler Adam T; Shan Xiaopeng; Münck Eckard; Que Lawrence
A synthetic precedent for the [FeIV2(mu-O)2] diamond core proposed for methane monooxygenase intermediate Q.
Proceedings of the National Academy of Sciences of the United States of America 2007;104(52):20713-8.
2007: Company Anna; Gómez Laura; Güell Mireia; Ribas Xavi; Luis Josep M; Que Lawrence; Costas Miquel
Alkane hydroxylation by a nonheme iron catalyst that challenges the heme paradigm for oxygenase action.
Journal of the American Chemical Society 2007;129(51):15766-7.
2007: Decker Andrea; Rohde Jan-Uwe; Klinker Eric J; Wong Shaun D; Que Lawrence; Solomon Edward I
Spectroscopic and quantum chemical studies on low-spin FeIV=O complexes: Fe-O bonding and its contributions to reactivity.
Journal of the American Chemical Society 2007;129(51):15983-96.
2007: Mas-Ballesté Rubén; Que Lawrence
Iron-catalyzed olefin epoxidation in the presence of acetic acid: insights into the nature of the metal-based oxidant.
Journal of the American Chemical Society 2007;129(51):15964-72.
2007: Sastri Chivukula V; Lee Jimin; Oh Kyungeun; Lee Yoon Jin; Lee Junghyun; Jackson Timothy A; Ray Kallol; Hirao Hajime; Shin Woonsup; Halfen Jason A; Kim Jinheung; Que Lawrence; Shaik Sason; Nam Wonwoo
Axial ligand tuning of a nonheme iron(IV)-oxo unit for hydrogen atom abstraction.
Proceedings of the National Academy of Sciences of the United States of America 2007;104(49):19181-6.
2007: Shan Xiaopeng; Rohde Jan-Uwe; Koehntop Kevin D; Zhou Yuming; Bukowski Michael R; Costas Miquel; Fujisawa Kiyoshi; Que Lawrence
X-ray absorption spectroscopic studies of high-spin nonheme (alkylperoxo)iron(III) intermediates.
Inorganic chemistry 2007;46(20):8410-7.
2007: Que Lawrence
The road to non-heme oxoferryls and beyond.
Accounts of chemical research 2007;40(7):493-500.
2007: Rohde Jan-Uwe; Betley Theodore A; Jackson Timothy A; Saouma Caroline T; Peters Jonas C; Que Lawrence
XAS characterization of a nitridoiron(IV) complex with a very short Fe-N bond.
Inorganic chemistry 2007;46(14):5720-6.
2007: Company Anna; Gómez Laura; Mas-Ballesté Rubén; Korendovych Ivan V; Ribas Xavi; Poater Albert; Parella Teodor; Fontrodona Xavier; Benet-Buchholz Jordi; Solà Miquel; Que Lawrence; Rybak-Akimova Elena V; Costas Miquel
Fast O2 binding at dicopper complexes containing Schiff-base dinucleating ligands.
Inorganic chemistry 2007;46(12):4997-5012.
2007: Klotz Katie L; Slominski Luke M; Hull Anthony V; Gottsacker Victoria M; Mas-Ballesté Rubén; Que Lawrence; Halfen Jason A
Non-heme iron(II) complexes are efficient olefin aziridination catalysts.
Chemical communications (Cambridge, England) 2007;(20):2063-5.
2007: Jensen Michael P; Payeras Antoni Mairata I; Fiedler Adam T; Costas Miquel; Kaizer József; Stubna Audria; Münck Eckard; Que Lawrence
Kinetic analysis of the conversion of nonheme (alkylperoxo)iron(III) species to iron(IV) complexes.
Inorganic chemistry 2007;46(7):2398-408.
2007: Tiago de Oliveira Filipe; Chanda Arani; Banerjee Deboshri; Shan Xiaopeng; Mondal Sujit; Que Lawrence; Bominaar Emile L; Münck Eckard; Collins Terrence J
Chemical and spectroscopic evidence for an FeV-oxo complex.
Science (New York, N.Y.) 2007;315(5813):835-8.
2007: Paine Tapan Kanti; England Jason; Que Lawrence
Iron-catalyzed C2-C3 bond cleavage of phenylpyruvate with O2: insight into aliphatic C-C bond-cleaving dioxygenases.
Chemistry (Weinheim an der Bergstrasse, Germany) 2007;13(21):6073-81.
2006: Oldenburg Paul D; Ke Chun-Yen; Tipton A Alex; Shteinman Albert A; Que Lawrence
A structural and functional model for dioxygenases with a 2-His-1-carboxylate triad.
Angewandte Chemie (International ed. in English) 2006;45(47):7975-8.
2006: Klinker Eric J; Jackson Timothy A; Jensen Michael P; Stubna Audria; Juhász Gergely; Bominaar Emile L; Münck Eckard; Que Lawrence
A tosylimido analogue of a nonheme oxoiron(IV) complex.
Angewandte Chemie (International ed. in English) 2006;45(44):7394-7.
2006: Collins Michael J; Ray Kallol; Que Lawrence
electrochemical generation of a nonheme oxoiron(IV) complex.
Inorganic chemistry 2006;45(20):8009-11.
2006: Klein David P; Young Victor G; Tolman William B; Que Lawrence
Mononitrosyl iron complexes supported by sterically hindered carboxylate ligands.
Inorganic chemistry 2006;45(20):8006-8.
2006: Friese Seth J; Kucera Benjamin E; Que Lawrence; Tolman William B
Self-assembly of the 2-His-1-carboxylate facial triad in mononuclear iron(II) and zinc(II) models of metalloenzyme active sites.
Inorganic chemistry 2006;45(20):8003-5.
2006: Mehn Mark P; Brown Steven D; Jenkins David M; Peters Jonas C; Que Lawrence
Vibrational spectroscopy and analysis of pseudo-tetrahedral complexes with metal imido bonds.
Inorganic chemistry 2006;45(18):7417-27.
2006: Bautz Jochen; Comba Peter; Que Lawrence
Spin-crossover in an iron(III)-bispidine-alkylperoxide system.
Inorganic chemistry 2006;45(18):7077-82.
2006: Mas-Ballesté Rubén; Costas Miquel; van den Berg Tieme; Que Lawrence
Ligand topology effects on olefin oxidations by bio-inspired [FeII(N2Py2)] catalysts.
Chemistry (Weinheim an der Bergstrasse, Germany) 2006;12(28):7489-500.
2006: Rohde Jan-Uwe; Stubna Audria; Bominaar Emile L; Münck Eckard; Nam Wonwoo; Que Lawrence
Nonheme oxoiron(IV) complexes of tris(2-pyridylmethyl)amine with cis-monoanionic ligands.
Inorganic chemistry 2006;45(16):6435-45.
2006: Bautz Jochen; Bukowski Michael R; Kerscher Marion; Stubna Audria; Comba Peter; Lienke Achim; Münck Eckard; Que Lawrence
Formation of an aqueous oxoiron(IV) complex at pH 2-6 from a nonheme iron(II) complex and H2O2.
Angewandte Chemie (International ed. in English) 2006;45(34):5681-4.
2006: Jensen Michael P; Que Emily L; Shan Xiaopeng; Rybak-Akimova Elena; Que Lawrence
Spectroscopic and kinetic studies of the reaction of [CuI(6-PhTPA)]+ with O2.
Dalton transactions (Cambridge, England : 2003) 2006;(29):3523-7.
2006: Company Anna; Lamata Diana; Poater Albert; Solà Miquel; Rybak-Akimova Elena V; Que Lawrence; Fontrodona Xavier; Parella Teodor; Llobet Antoni; Costas Miquel
O2 chemistry of dicopper complexes with alkyltriamine ligands. Comparing synergistic effects on O2 binding.
Inorganic chemistry 2006;45(14):5239-41.
2006: Mas-Ballesté Rubén; Que Lawrence
Chemistry. Targeting specific C-H bonds for oxidation.
Science (New York, N.Y.) 2006;312(5782):1885-6.
2006: Bukowski Michael R; Comba Peter; Lienke Achim; Limberg Christian; Lopez de Laorden Carlos; Mas-Ballesté Rubén; Merz Michael; Que Lawrence
Catalytic epoxidation and 1,2-dihydroxylation of olefins with bispidine-iron(II)/H2O2 systems.
Angewandte Chemie (International ed. in English) 2006;45(21):3446-9.
2006: Paine Tapan K; Costas Miquel; Kaizer József; Que Lawrence
Oxoiron(IV) complexes of the tris(2-pyridylmethyl)amine ligand family: effect of pyridine alpha-substituents.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2006;11(3):272-6.
2006: Shan Xiaopeng; Que Lawrence
High-valent nonheme iron-oxo species in biomimetic oxidations.
Journal of inorganic biochemistry 2006;100(4):421-33.
2006: Mehn Mark P; Brown Steven D; Paine Tapan K; Brennessel William W; Cramer Christopher J; Peters Jonas C; Que Lawrence
High-spin and low-spin iron(II) complexes with facially-coordinated borohydride ligands.
Dalton transactions (Cambridge, England : 2003) 2006;(10):1347-51.
2006: Koehntop Kevin D; Marimanikkuppam Sudha; Ryle Matthew J; Hausinger Robert P; Que Lawrence
Self-hydroxylation of taurine/alpha-ketoglutarate dioxygenase: evidence for more than one oxygen activation mechanism.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2006;11(1):63-72.
2005: Oh Na Young; Seo Mi Sook; Lim Mi Hee; Consugar Mark B; Park Mi Joo; Rohde Jan-Uwe; Han Jaehong; Kim Kwan Mook; Kim Jinheung; Que Lawrence; Nam Wonwoo
Self-hydroxylation of perbenzoic acids at a nonheme iron(II) center.
Chemical communications (Cambridge, England) 2005;(45):5644-6.
2005: Earhart Cathleen A; Vetting Matthew W; Gosu Ramachandraiah; Michaud-Soret Isabelle; Que Lawrence; Ohlendorf Douglas H
Structure of catechol 1,2-dioxygenase from Pseudomonas arvilla.
Biochemical and biophysical research communications 2005;338(1):198-205.
2005: Farquhar Erik R; Koehntop Kevin D; Emerson Joseph P; Que Lawrence
Post-translational self-hydroxylation: a probe for oxygen activation mechanisms in non-heme iron enzymes.
Biochemical and biophysical research communications 2005;338(1):230-9.
2005: Oldenburg Paul D; Shteinman Albert A; Que Lawrence
Iron-catalyzed olefin cis-dihydroxylation using a bio-inspired N,N,O-ligand.
Journal of the American Chemical Society 2005;127(45):15672-3.
2005: Bukowski Michael R; Koehntop Kevin D; Stubna Audria; Bominaar Emile L; Halfen Jason A; Münck Eckard; Nam Wonwoo; Que Lawrence
A thiolate-ligated nonheme oxoiron(IV) complex relevant to cytochrome P450.
Science (New York, N.Y.) 2005;310(5750):1000-2.
2005: Taktak Sonia; Flook Margaret; Foxman Bruce M; Que Lawrence; Rybak-Akimova Elena V
Ortho-hydroxylation of benzoic acids with hydrogen peroxide at a non-heme iron center.
Chemical communications (Cambridge, England) 2005;(42):5301-3.
2005: Emerson Joseph P; Wagner Michelle L; Reynolds Mark F; Que Lawrence; Sadowsky Michael J; Wackett Lawrence P
The role of histidine 200 in MndD, the Mn(II)-dependent 3,4-dihydroxyphenylacetate 2,3-dioxygenase from Arthrobacter globiformis CM-2, a site-directed mutagenesis study.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2005;10(7):751-60.
2005: Pestovsky Oleg; Stoian Sebastian; Bominaar Emile L; Shan Xiaopeng; Münck Eckard; Que Lawrence; Bakac Andreja
Aqueous FeIV==O: spectroscopic identification and oxo-group exchange.
Angewandte Chemie (International ed. in English) 2005;44(42):6871-4.
2005: Sastri Chivukula V; Park Mi Joo; Ohta Takehiro; Jackson Timothy A; Stubna Audria; Seo Mi Sook; Lee Jimin; Kim Jinheung; Kitagawa Teizo; Münck Eckard; Que Lawrence; Nam Wonwoo
Axial ligand substituted nonheme FeIV=O complexes: observation of near-UV LMCT bands and Fe=O Raman vibrations.
Journal of the American Chemical Society 2005;127(36):12494-5.
2005: Jensen Michael P; Costas Miquel; Ho Raymond Y N; Kaizer József; Mairata i Payeras Antoni; Münck Eckard; Que Lawrence; Rohde Jan-Uwe; Stubna Audria
High-valent nonheme iron. Two distinct iron(IV) species derived from a common iron(II) precursor.
Journal of the American Chemical Society 2005;127(30):10512-25.
2005: Klinker Eric J; Kaizer József; Brennessel William W; Woodrum Nathaniel L; Cramer Christopher J; Que Lawrence
Structures of nonheme oxoiron(IV) complexes from X-ray crystallography, NMR spectroscopy, and DFT calculations.
Angewandte Chemie (International ed. in English) 2005;44(24):3690-4.
2005: Tierney David L; Rocklin Amy M; Lipscomb John D; Que Lawrence; Hoffman Brian M
ENDOR studies of the ligation and structure of the non-heme iron site in ACC oxidase.
Journal of the American Chemical Society 2005;127(19):7005-13.
2005: Quiñonero David; Morokuma Keiji; Musaev Djamaladdin G; Mas-Ballesté Rubén; Que Lawrence
Metal-peroxo versus metal-oxo oxidants in non-heme iron-catalyzed olefin oxidations: computational and experimental studies on the effect of water.
Journal of the American Chemical Society 2005;127(18):6548-9.
2005: Shan Xiaopeng; Que Lawrence
Intermediates in the oxygenation of a nonheme diiron(II) complex, including the first evidence for a bound superoxo species.
Proceedings of the National Academy of Sciences of the United States of America 2005;102(15):5340-5.
2005: Rohde Jan-Uwe; Que Lawrence
Axial coordination of carboxylate activates the non-heme FeIV=O unit.
Angewandte Chemie (International ed. in English) 2005;44(15):2255-8.
2005: Koehntop Kevin D; Emerson Joseph P; Que Lawrence
The 2-His-1-carboxylate facial triad: a versatile platform for dioxygen activation by mononuclear non-heme iron(II) enzymes.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2005;10(2):87-93.
2005: Paine Tapan K; Zheng Hui; Que Lawrence
Iron Coordination Chemistry of Phenylpyruvate: An Unexpected kappa3-bridging mode that leads to oxidative cleavage of the C2-C3 bond.
Inorganic chemistry 2005;44(3):474-6.
2005: Kryatov Sergey V; Taktak Sonia; Korendovych Ivan V; Rybak-Akimova Elena V; Kaizer József; Torelli Stéphane; Shan Xiaopeng; Mandal Sanjay; MacMurdo Vicki L; Mairata i Payeras Antoni; Que Lawrence
Dioxygen binding to complexes with Fe(II)2(mu-OH)2 cores: steric control of activation barriers and O2-adduct formation.
Inorganic chemistry 2005;44(1):85-99.
2005: Bukowski Michael R; Halfen Heather L; van den Berg Tieme A; Halfen Jason A; Que Lawrence
Spin-state rationale for the peroxo-stabilizing role of the thiolate ligand in superoxide reductase.
Angewandte Chemie (International ed. in English) 2005;44(4):584-7.
2004: Rohde Jan-Uwe; Torelli Stéphane; Shan Xiaopeng; Lim Mi Hee; Klinker Eric J; Kaizer József; Chen Kui; Nam Wonwoo; Que Lawrence
Structural insights into nonheme alkylperoxoiron(III) and oxoiron(IV) intermediates by X-ray absorption spectroscopy.
Journal of the American Chemical Society 2004;126(51):16750-61.
2004: Koehntop Kevin D; Rohde Jan-Uwe; Costas Miquel; Que Lawrence
XAS characterization of end-on and side-on peroxoiron(III) complexes of the neutral pentadentate N-donor ligand N-methyl-N,N',N'-tris(2-pyridylmethyl)ethane-1,2-diamine.
Dalton transactions (Cambridge, England : 2003) 2004;(20):3191-8.
2004: Mairata i Payeras Antoni; Ho Raymond Y N; Fujita Megumi; Que Lawrence
The reaction of [FeII(tpa)] with H2O2 in acetonitrile and acetone--distinct intermediates and yet similar catalysis.
Chemistry (Weinheim an der Bergstrasse, Germany) 2004;10(20):4944-53.
2004: Que Lawrence
The heme paradigm revisited: alternative reaction pathways considered.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2004;9(6):643.
2004: Que Lawrence
The oxo/peroxo debate: a nonheme iron perspective.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2004;9(6):684-90.
2004: Liu Pinghua; Mehn Mark P; Yan Feng; Zhao Zongbao; Que Lawrence; Liu Hung-wen
Oxygenase activity in the self-hydroxylation of (s)-2-hydroxypropylphosphonic acid epoxidase involved in fosfomycin biosynthesis.
Journal of the American Chemical Society 2004;126(33):10306-12.
2004: Stubna Audria; Jo Du-Hwan; Costas Miquel; Brenessel William W; Andres Hanspeter; Bominaar Emile L; Münck Eckard; Que Lawrence
A structural and Mössbauer study of complexes with Fe(2)(micro-O(H))(2) cores: stepwise oxidation from Fe(II)(micro-OH)(2)Fe(II) through Fe(II)(micro-OH)(2)Fe(III) to Fe(III)(micro-O)(micro-OH)Fe(III).
Inorganic chemistry 2004;43(10):3067-79.
2004: Decker Andrea; Rohde Jan-Uwe; Que Lawrence; Solomon Edward I
Spectroscopic and quantum chemical characterization of the electronic structure and bonding in a non-heme FeIV[double bond]O complex.
Journal of the American Chemical Society 2004;126(17):5378-9.
2004: Seo Mi Sook; In Jun-Hee; Kim Sun Ok; Oh Na Young; Hong Jongki; Kim Jinheung; Que Lawrence; Nam Wonwoo
Direct evidence for oxygen-atom exchange between nonheme oxoiron(IV) complexes and isotopically labeled water.
Angewandte Chemie (International ed. in English) 2004;43(18):2417-20.
2004: Vetting Matthew W; Wackett Lawrence P; Que Lawrence; Lipscomb John D; Ohlendorf Douglas H
Crystallographic comparison of manganese- and iron-dependent homoprotocatechuate 2,3-dioxygenases.
Journal of bacteriology 2004;186(7):1945-58.
2004: Zlateva Theodora; Quaroni Luca; Que Lawrence; Stankovich Marian T
Redox studies of subunit interactivity in aerobic ribonucleotide reductase from Escherichia coli.
The Journal of biological chemistry 2004;279(18):18742-7.
2004: Kryatov Sergey V; Chavez Ferman A; Reynolds Anne M; Rybak-Akimova Elena V; Que Lawrence; Tolman William B
Mechanistic studies on the formation and reactivity of dioxygen adducts of diiron complexes supported by sterically hindered carboxylates.
Inorganic chemistry 2004;43(6):2141-50.
2004: Rocklin Amy M; Kato Keisuke; Liu Hung-wen; Que Lawrence; Lipscomb John D
Mechanistic studies of 1-aminocyclopropane-1-carboxylic acid oxidase: single turnover reaction.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2004;9(2):171-82.
2004: Bukowski Michael R; Comba Peter; Limberg Christian; Merz Michael; Que Lawrence; Wistuba Tobias
Bispidine ligand effects on iron/hydrogen peroxide chemistry.
Angewandte Chemie (International ed. in English) 2004;43(10):1283-7.
2004: Costas Miquel; Mehn Mark P; Jensen Michael P; Que Lawrence
Dioxygen activation at mononuclear nonheme iron active sites: enzymes, models, and intermediates.
Chemical reviews 2004;104(2):939-86.
2004: Kaizer József; Klinker Eric J; Oh Na Young; Rohde Jan-Uwe; Song Woon Ju; Stubna Audria; Kim Jinheung; Münck Eckard; Nam Wonwoo; Que Lawrence
Nonheme FeIVO complexes that can oxidize the C-H bonds of cyclohexane at room temperature.
Journal of the American Chemical Society 2004;126(2):472-3.
2004: Bukowski Michael R; Zhu Shourong; Koehntop Kevin D; Brennessel William W; Que Lawrence
Characterization of an Fe III-OOH species and its decomposition product in a bleomycin model system.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2004;9(1):39-48.
2003: Rohde Jan-Uwe; Bukowski Michael R; Que Lawrence
Functional models for mononuclear nonheme iron enzymes.
Current opinion in chemical biology 2003;7(6):674-82.
2003: Costas Miquel; Cady Clyde W; Kryatov Sergey V; Ray Manabendra; Ryan Meghan J; Rybak-Akimova Elena V; Que Lawrence
Role of carboxylate bridges in modulating nonheme diiron(II)/O(2) reactivity.
Inorganic chemistry 2003;42(23):7519-30.
2003: Skulan Andrew J; Hanson Melissa A; Hsu Hua-fen; Dong Yanhong; Que Lawrence; Solomon Edward I
EPR spectroscopy of [Fe2O2(5-Et3-TPA)2]3+: electronic origin of the unique spin-Hamiltonian parameters of the Fe2(III,IV)O2 diamond core.
Inorganic chemistry 2003;42(20):6489-96.
2003: Jensen Michael P; Mehn Mark P; Que Lawrence
Intramolecular aromatic amination through iron-mediated nitrene transfer.
Angewandte Chemie (International ed. in English) 2003;42(36):4357-60.
2003: Kaizer József; Costas Miquel; Que Lawrence
A dramatic push effect on the homolysis of FeIII(OOR) intermediates to form non-heme FeIV=O complexes.
Angewandte Chemie (International ed. in English) 2003;42(31):3671-3.
2003: Fujita Megumi; Costas Miquel; Que Lawrence
Iron-catalyzed olefin cis-dihydroxylation by H2O2: electrophilic versus nucleophilic mechanisms.
Journal of the American Chemical Society 2003;125(33):9912-3.
2003: Mehn Mark P; Fujisawa Kiyoshi; Hegg Eric L; Que Lawrence
Oxygen activation by nonheme iron(II) complexes: alpha-keto carboxylate versus carboxylate.
Journal of the American Chemical Society 2003;125(26):7828-42.
2003: Skulan Andrew J; Hanson Melissa A; Hsu Hua-Fen; Que Lawrence; Solomon Edward I
Spectroscopic study of [Fe2O2(5-Et3-TPA)2]3+: nature of the Fe2O2 diamond core and its possible relevance to high-valent binuclear non-heme enzyme intermediates.
Journal of the American Chemical Society 2003;125(24):7344-56.
2003: Roelfes Gerard; Vrajmasu Vladislav; Chen Kui; Ho Raymond Y N; Rohde Jan-Uwe; Zondervan Charon; La Crois Rene M; Schudde Ebe P; Lutz Martin; Spek Anthony L; Hage Ronald; Feringa Ben L; Münck Eckard; Que Lawrence
End-on and side-on peroxo derivatives of non-heme iron complexes with pentadentate ligands: models for putative intermediates in biological iron/dioxygen chemistry.
Inorganic chemistry 2003;42(8):2639-53.
2003: Lim Mi Hee; Rohde Jan-Uwe; Stubna Audria; Bukowski Michael R; Costas Miquel; Ho Raymond Y N; Munck Eckard; Nam Wonwoo; Que Lawrence
An FeIV=O complex of a tetradentate tripodal nonheme ligand.
Proceedings of the National Academy of Sciences of the United States of America 2003;100(7):3665-70.
2003: Ryle Matthew J; Koehntop Kevin D; Liu Aimin; Que Lawrence; Hausinger Robert P
Interconversion of two oxidized forms of taurine/alpha-ketoglutarate dioxygenase, a non-heme iron hydroxylase: evidence for bicarbonate binding.
Proceedings of the National Academy of Sciences of the United States of America 2003;100(7):3790-5.
2003: Ryle Matthew J; Liu Aimin; Muthukumaran Rajendra Bose; Ho Raymond Y N; Koehntop Kevin D; McCracken John; Que Lawrence; Hausinger Robert P
O2- and alpha-ketoglutarate-dependent tyrosyl radical formation in TauD, an alpha-keto acid-dependent non-heme iron dioxygenase.
Biochemistry 2003;42(7):1854-62.
2003: Jensen Michael P; Lange Steven J; Mehn Mark P; Que Emily L; Que Lawrence
Biomimetic aryl hydroxylation derived from alkyl hydroperoxide at a nonheme iron center. Evidence for an Fe(IV)=O oxidant.
Journal of the American Chemical Society 2003;125(8):2113-28.
2003: Reynolds Mark F; Costas Miquel; Ito Masami; Jo Du-Hwan; Tipton A Alex; Whiting Adam K; Que Lawrence
4-nitrocatechol as a probe of a Mn(II)-dependent extradiol-cleaving catechol dioxygenase (MndD): comparison with relevant Fe(II) and Mn(II) model complexes.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2003;8(3):263-72.
2003: Rohde Jan-Uwe; In Jun-Hee; Lim Mi Hee; Brennessel William W; Bukowski Michael R; Stubna Audria; Münck Eckard; Nam Wonwoo; Que Lawrence
Crystallographic and spectroscopic characterization of a nonheme Fe(IV)-O complex.
Science (New York, N.Y.) 2003;299(5609):1037-9.
2003: Nam Wonwoo; Choi Sun Kyung; Lim Mi Hee; Rohde Jan-Uwe; Kim Inwoo; Kim Jinheung; Kim Cheal; Que Lawrence
Reversible formation of iodosylbenzene-iron porphyrin intermediates in the reaction of oxoiron(IV) porphyrin pi-cation radicals and iodobenzene.
Angewandte Chemie (International ed. in English) 2003;42(1):109-11.
2002: Lehnert Nicolai; Neese Frank; Ho Raymond Y N; Que Lawrence; Solomon Edward I
Electronic structure and reactivity of low-spin Fe(III)-hydroperoxo complexes: comparison to activated bleomycin.
Journal of the American Chemical Society 2002;124(36):10810-22.
2002: Costas Miquel; Que Lawrence
Ligand topology tuning of iron-catalyzed hydrocarbon oxidations.
Angewandte Chemie (International ed. in English) 2002;41(12):2179-81.
2002: Ryu Ju Yeon; Kim Jinheung; Costas Miquel; Chen Kui; Nam Wonwoo; Que Lawrence
High conversion of olefins to cis-diols by non-heme iron catalysts and H2O2.
Chemical communications (Cambridge, England) 2002;(12):1288-9.
2002: Zhou Jing; Rocklin Amy M; Lipscomb John D; Que Lawrence; Solomon Edward I
Spectroscopic studies of 1-aminocyclopropane-1-carboxylic acid oxidase: molecular mechanism and CO(2) activation in the biosynthesis of ethylene.
Journal of the American Chemical Society 2002;124(17):4602-9.
2002: Que Lawrence; Tolman William B
Bis(mu-oxo)dimetal "diamond" cores in copper and iron complexes relevant to biocatalysis.
Angewandte Chemie (International ed. in English) 2002;41(7):1114-37.
2002: Chen Kui; Costas Miquel; Kim Jinheung; Tipton Adrianne K; Que Lawrence
Olefin cis-dihydroxylation versus epoxidation by non-heme iron catalysts: two faces of an Fe(III)-OOH coin.
Journal of the American Chemical Society 2002;124(12):3026-35.
2002: Mekmouche Yasmina; Hummel Helga; Ho Raymond Y N; Que Lawrence; Schünemann Volker; Thomas Fabrice; Trautwein Alfred X; Lebrun Colette; Gorgy Karine; Leprêtre Jean-Claude; Collomb Marie-Noëlle; Deronzier Alain; Fontecave Marc; Ménage Stéphane
Sulfide oxidation by hydrogen peroxide catalyzed by iron complexes: two metal centers are better than one.
Chemistry (Weinheim an der Bergstrasse, Germany) 2002;8(5):1196-204.
2002: Chavez Ferman A; Ho Raymond Y N; Pink Maren; Young Victor G; Kryatov Sergei V; Rybak-Akimova Elena V; Andres Hanspeter; Münck Eckard; Que Lawrence; Tolman William B
Unusual peroxo intermediates in the reaction of dioxygen with carboxylate-bridged diiron(II,II) paddlewheel complexes.
Angewandte Chemie (International ed. in English) 2002;41(1):149-52.
2001: Costas M; Rohde J U; Stubna A; Ho R Y; Quaroni L; Münck E; Que L
A synthetic model for the putative Fe(IV)(2)O(2) diamond core of methane monooxygenase intermediate Q.
Journal of the American Chemical Society 2001;123(51):12931-2.
2001: Lehnert N; Ho R Y; Que L; Solomon E I
Electronic structure of high-spin iron(III)-alkylperoxo complexes and its relation to low-spin analogues: reaction coordinate of O-O bond homolysis.
Journal of the American Chemical Society 2001;123(51):12802-16.
2001: Halfen J A; Fox D C; Mehn M P; Que L
Enhanced reactivity of copper catalysts for olefin aziridination by manipulation of ligand denticity.
Inorganic chemistry 2001;40(20):5060-1.
2001: Lehnert N; Ho R Y; Que L; Solomon E I
Spectroscopic properties and electronic structure of low-spin Fe(III)-alkylperoxo complexes: homolytic cleavage of the O-O bond.
Journal of the American Chemical Society 2001;123(34):8271-90.
2001: Chen K; Que L
Stereospecific alkane hydroxylation by non-heme iron catalysts: mechanistic evidence for an Fe(V)=O active species.
Journal of the American Chemical Society 2001;123(26):6327-37.
2001: Miyake H; Chen K; Lange S J; Que L
"Intermolecular" trapping of a nonheme Fe(IV)=O intermediate.
Inorganic chemistry 2001;40(14):3534-8.
2001: Jo D H; Chiou Y M; Que L
Models for extradiol cleaving catechol dioxygenases: syntheses, structures, and reactivities of iron(II)-monoanionic catecholate complexes.
Inorganic chemistry 2001;40(13):3181-90.
2001: Liu A; Ho R Y; Que L; Ryle M J; Phinney B S; Hausinger R P
Alternative reactivity of an alpha-ketoglutarate-dependent iron(II) oxygenase: enzyme self-hydroxylation.
Journal of the American Chemical Society 2001;123(21):5126-7.
2001: Ho R Y; Mehn M P; Hegg E L; Liu A; Ryle M J; Hausinger R P; Que L
Resonance Raman studies of the iron(II)--alpha-keto acid chromophore in model and enzyme complexes.
Journal of the American Chemical Society 2001;123(21):5022-9.
2001: Kryatov S V; Rybak-Akimova E V; MacMurdo V L; Que L
A mechanistic study of the reaction between a diiron(II) complex [FeII(2)(mu-OH)2(6-Me3-TPA)2](2+) and O2 to form a diiron(III) peroxo complex.
Inorganic chemistry 2001;40(10):2220-8.
2001: Branum M E; Tipton A K; Zhu S; Que L
Double-strand hydrolysis of plasmid DNA by dicerium complexes at 37 degrees C.
Journal of the American Chemical Society 2001;123(9):1898-904.
2001: Kim J; Zang Y; Costas M; Harrison R G; Wilkinson E C; Que L
A nonheme iron(II) complex that models the redox cycle of lipoxygenase.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 2001;6(3):275-84.
2000: Halfen J A; Uhan J M; Fox D C; Mehn M P; Que L
Copper(II) complexes of pyridyl-appended diazacycloalkanes: synthesis, characterization, and application to catalytic olefin aziridination.
Inorganic chemistry 2000;39(21):4913-20.
2000: MacMurdo V L; Zheng H; Que L
Model for the cofactor formation reaction of E. coli ribonucleotide reductase. From a diiron(II) precursor to an FeIIIFeIV species via a peroxo intermediate.
Inorganic chemistry 2000;39(11):2254-5.
2000: Mandal S K; Young V G; Que L
Polynuclear carboxylato-bridged iron(II) clusters: synthesis, structure, and host-guest chemistry.
Inorganic chemistry 2000;39(8):1831-3.
1999: Hegg E L; Whiting A K; Saari R E; McCracken J; Hausinger R P; Que L
Herbicide-degrading alpha-keto acid-dependent enzyme TfdA: metal coordination environment and mechanistic insights.
Biochemistry 1999;38(50):16714-26.
1999: Branum M E; Que L
Double-strand DNA hydrolysis by dilanthanide complexes.
Journal of biological inorganic chemistry : JBIC : a publication of the Society of Biological Inorganic Chemistry 1999;4(5):593-600.
1999: Rocklin A M; Tierney D L; Kofman V; Brunhuber N M; Hoffman B M; Christoffersen R E; Reich N O; Lipscomb J D; Que L
Role of the nonheme Fe(II) center in the biosynthesis of the plant hormone ethylene.
Proceedings of the National Academy of Sciences of the United States of America 1999;96(14):7905-9.
1997: Hegg E L; Que L
The 2-His-1-carboxylate facial triad--an emerging structural motif in mononuclear non-heme iron(II) enzymes.
European journal of biochemistry / FEBS 1997;250(3):625-9.
1997: Lehmann T E; Ming L J; Rosen M E; Que L
NMR studies of the paramagnetic complex Fe(II)-bleomycin.
Biochemistry 1997;36(10):2807-16.
1997: Boldt Y R; Whiting A K; Wagner M L; Sadowsky M J; Que L; Wackett L P
Manganese(II) active site mutants of 3,4-dihydroxyphenylacetate 2,3-dioxygenase from Arthrobacter globiformis strain CM-2.
Biochemistry 1997;36(8):2147-53.
1997: Shu L; Nesheim J C; Kauffmann K; Münck E; Lipscomb J D; Que L
An Fe2IVO2 diamond core structure for the key intermediate Q of methane monooxygenase.
Science (New York, N.Y.) 1997;275(5299):515-8.
1996: Wang X; Randall C R; True A E; Que L
X-ray absorption spectroscopic studies of the FeZn derivative of uteroferrin.
Biochemistry 1996;35(44):13946-54.
1996: Halfen J A; Mahapatra S; Wilkinson E C; Kaderli S; Young V G; Que L; Zuberbühler A D; Tolman W B
Reversible cleavage and formation of the dioxygen O-O bond within a dicopper complex.
Science (New York, N.Y.) 1996;271(5254):1397-400.
1996: Whiting A K; Boldt Y R; Hendrich M P; Wackett L P; Que L
Manganese(II)-dependent extradiol-cleaving catechol dioxygenase from Arthrobacter globiformis CM-2.
Biochemistry 1996;35(1):160-70.
1995: Silva K E; Elgren T E; Que L; Stankovich M T
Electron transfer properties of the R2 protein of ribonucleotide reductase from Escherichia coli.
Biochemistry 1995;34(43):14093-103.
1995: Haskin C J; Ravi N; Lynch J B; Münck E; Que L
Reaction of NO with the reduced R2 protein of ribonucleotide reductase from Escherichia coli.
Biochemistry 1995;34(35):11090-8.
1995: Shu L; Chiou Y M; Orville A M; Miller M A; Lipscomb J D; Que L
X-ray absorption spectroscopic studies of the Fe(II) active site of catechol 2,3-dioxygenase. Implications for the extradiol cleavage mechanism.
Biochemistry 1995;34(20):6649-59.
1995: Michaud-Soret I; Andersson K K; Que L; Haavik J
Resonance Raman studies of catecholate and phenolate complexes of recombinant human tyrosine hydroxylase.
Biochemistry 1995;34(16):5504-10.
1995: Boldt Y R; Sadowsky M J; Ellis L B; Que L; Wackett L P
A manganese-dependent dioxygenase from Arthrobacter globiformis CM-2 belongs to the major extradiol dioxygenase family.
Journal of bacteriology 1995;177(5):1225-32.
1994: Earhart C A; Hall M D; Michaud-Soret I; Que L; Ohlendorf D H
Crystallization of catechol-1,2 dioxygenase from Pseudomonas arvilla C-1.
Journal of molecular biology 1994;236(1):377-8.
1994: Schnaith L M; Hanson R S; Que L
Double-stranded cleavage of pBR322 by a diiron complex via a "hydrolytic" mechanism.
Proceedings of the National Academy of Sciences of the United States of America 1994;91(2):569-73.
1993: Randall C R; Zang Y; True A E; Que L; Charnock J M; Garner C D; Fujishima Y; Schofield C J; Baldwin J E
X-ray absorption studies of the ferrous active site of isopenicillin N synthase and related model complexes.
Biochemistry 1993;32(26):6664-73.
1992: Crans D C; Simone C M; Holz R C; Que L
Interaction of porcine uterine fluid purple acid phosphatase with vanadate and vanadyl cation.
Biochemistry 1992;31(47):11731-9.
1992: Siu D C; Orville A M; Lipscomb J D; Ohlendorf D H; Que L
Resonance Raman studies of the protocatechuate 3,4-dioxygenase from Brevibacterium fuscum.
Biochemistry 1992;31(43):10443-8.
1992: Olson P E; Qi B; Que L; Wackett L P
Immunological demonstration of a unique 3,4-dihydroxyphenylacetate 2,3-dioxygenase in soil Arthrobacter strains.
Applied and environmental microbiology 1992;58(9):2820-6.
1992: Wang Z; Ming L J; Que L; Vincent J B; Crowder M W; Averill B A
1H NMR and NOE studies of the purple acid phosphatases from porcine uterus and bovine spleen.
Biochemistry 1992;31(23):5263-8.
1992: Andersson K K; Vassort C; Brennan B A; Que L; Haavik J; Flatmark T; Gros F; Thibault J
Purification and characterization of the blue-green rat phaeochromocytoma (PC12) tyrosine hydroxylase with a dopamine-Fe(III) complex. Reversal of the endogenous feedback inhibition by phosphorylation of serine-40.
The Biochemical journal 1992;284 ( Pt 3)():687-95.
1991: Ming L J; Que L; Kriauciunas A; Frolik C A; Chen V J
NMR studies of the active site of isopenicillin N synthase, a non-heme iron(II) enzyme.
Biochemistry 1991;30(50):11653-9.
1991: Jiang F; Peisach J; Ming L J; Que L; Chen V J
Electron spin echo envelope modulation studies of the Cu(II)-substituted derivative of isopenicillin N synthase: a structural and spectroscopic model.
Biochemistry 1991;30(48):11437-45.
1991: Elgren T E; Lynch J B; Juarez-Garcia C; Münck E; Sjöberg B M; Que L
Electron transfer associated with oxygen activation in the B2 protein of ribonucleotide reductase from Escherichia coli.
The Journal of biological chemistry 1991;266(29):19265-8.
1991: Wang D L; Holz R C; David S S; Que L; Stankovich M T
Electrochemical properties of the diiron core of uteroferrin and its anion complexes.
Biochemistry 1991;30(33):8187-94.
1991: Que L
Oxygen activation at the diiron center of ribonucleotide reductase.
Science (New York, N.Y.) 1991;253(5017):273-4.
1991: Hendrich M P; Elgren T E; Que L
A mixed valence form of the iron cluster in the B2 protein of ribonucleotide reductase from Escherichia coli.
Biochemical and biophysical research communications 1991;176(2):705-10.
1990: True A E; Orville A M; Pearce L L; Lipscomb J D; Que L
An EXAFS study of the interaction of substrate with the ferric active site of protocatechuate 3,4-dioxygenase.
Biochemistry 1990;29(48):10847-54.
1989: Lynch J B; Juarez-Garcia C; Münck E; Que L
Mössbauer and EPR studies of the binuclear iron center in ribonucleotide reductase from Escherichia coli. A new iron-to-protein stoichiometry.
The Journal of biological chemistry 1989;264(14):8091-6.
1988: Andersson K K; Cox D D; Que L; Flatmark T; Haavik J
Resonance Raman studies on the blue-green-colored bovine adrenal tyrosine 3-monooxygenase (tyrosine hydroxylase). Evidence that the feedback inhibitors adrenaline and noradrenaline are coordinated to iron.
The Journal of biological chemistry 1988;263(35):18621-6.
1988: Day E P; David S S; Peterson J; Dunham W R; Bonvoisin J J; Sands R H; Que L
Magnetization and electron paramagnetic resonance studies of reduced uteroferrin and its "EPR-silent" phosphate complex.
The Journal of biological chemistry 1988;263(30):15561-7.

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