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Eberhard Bothe

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Chemicals & Drugs

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Oxidation-Reduction

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Julia B H Strautmann; Carl-Georg Freiherr von Richthofen; Gabriele Heinze-Brückner; Serena DeBeer; Eberhard Bothe; Eckhard Bill; Thomas Weyhermüller; Anja Stammler; Hartmut Bögge; Thorsten Glaser
Molecular and electronic structures of dinuclear iron complexes incorporating strongly electron-donating ligands: implications for the generation of the one- and two-electron oxidized forms.
Julia Bernhardette Hildegard Strautmann; Carl-Georg Freiherr von Richthofen; Serena DeBeer George; Eberhard Bothe; Eckhard Bill; Thorsten Glaser
Highly oxidized diiron complexes: generation, spectroscopy, and stabilities.
Connie C Lu; Eckhard Bill; Thomas Weyhermüller; Eberhard Bothe; Karl Wieghardt
Neutral bis(alpha-iminopyridine)metal complexes of the first-row transition ions (Cr, Mn, Fe, Co, Ni, Zn) and their monocationic analogues: mixed valency involving a redox noninnocent ligand system.

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All Publications

2011: Julia B H Strautmann; Carl-Georg Freiherr von Richthofen; Gabriele Heinze-Brückner; Serena DeBeer; Eberhard Bothe; Eckhard Bill; Thomas Weyhermüller; Anja Stammler; Hartmut Bögge; Thorsten Glaser
Molecular and electronic structures of dinuclear iron complexes incorporating strongly electron-donating ligands: implications for the generation of the one- and two-electron oxidized forms.
Inorganic chemistry 2011;50(1):155-71.
2009: Julia Bernhardette Hildegard Strautmann; Carl-Georg Freiherr von Richthofen; Serena DeBeer George; Eberhard Bothe; Eckhard Bill; Thorsten Glaser
Highly oxidized diiron complexes: generation, spectroscopy, and stabilities.
Chemical communications (Cambridge, England) 2009;(19):2637-9.
2008: Connie C Lu; Eckhard Bill; Thomas Weyhermüller; Eberhard Bothe; Karl Wieghardt
Neutral bis(alpha-iminopyridine)metal complexes of the first-row transition ions (Cr, Mn, Fe, Co, Ni, Zn) and their monocationic analogues: mixed valency involving a redox noninnocent ligand system.
Journal of the American Chemical Society 2008;130(10):3181-97.
2008: Connie C Lu; Serena DeBeer George; Thomas Weyhermüller; Eckhard Bill; Eberhard Bothe; Karl Wieghardt
An electron-transfer series of high-valent chromium complexes with redox non-innocent, non-heme ligands.
Angewandte Chemie (International ed. in English) 2008;47(34):6384-7.
2008: Marat M Khusniyarov; Eckhard Bill; Thomas Weyhermüller; Eberhard Bothe; Klaus Harms; Jörg Sundermeyer; Karl Wieghardt
Characterization of three members of the electron-transfer series [Fe(pda)2]n (n=2-, 1-, 0) by spectroscopy and density functional theoretical calculations [pda=redox non-innocent derivatives of N,N'-bis(pentafluorophenyl)-o-phenylenediamide(2-, 1.-, 0)].
Chemistry (Weinheim an der Bergstrasse, Germany) 2008;14(25):7608-22.
2007: Chandan Mukherjee; Thomas Weyhermüller; Eberhard Bothe; Eva Rentschler; Phalguni Chaudhuri
A tetracopper(II)-tetraradical cuboidal core and its reactivity as a functional model of phenoxazinone synthase.
Inorganic chemistry 2007;46(23):9895-905.
2007: Laurent Benisvy; Deborah Hammond; David J Parker; E Stephen Davies; C David Garner; Jonathan McMaster; Claire Wilson; Frank Neese; Eberhard Bothe; Robert Bittl; Christian Teutloff
Insights into the nature of the hydrogen bonding of *Tyr272 in apo-galactose oxidase.
Journal of inorganic biochemistry 2007;101(11-12):1859-64.
2007: Phalguni Chaudhuri; Thomas Weyhermüller; Rita Wagner; Sumit Khanra; Biplab Biswas; Eberhard Bothe; Eckhard Bill
Tridentate facial ligation of tris(pyridine-2-aldoximato)nickel(II) and tris(imidazole-2-aldoximato)nickel(II) To generate NiIIFeIIINiII, MnIIINiII, NiIINiII, and ZnIINiII and the electrooxidized MnIVNiII, NiIINiIII, and ZnIINiIII species: a magnetostructural, electrochemical, and EPR spectroscopic study.
Inorganic chemistry 2007;46(21):9003-16.
2007: Ruta R Kapre; Eberhard Bothe; Thomas Weyhermüller; Serena DeBeer George; Nicoleta Muresan; Karl Wieghardt
Electronic structures of tris(dioxolene)chromium and tris(dithiolene)chromium complexes of the electron-transfer series [Cr(dioxolene)(3)](z) and [Cr(dithiolene)(3)](z) (z = 0, 1-, 2-, 3-). A combined experimental and density functional theoretical study.
Inorganic chemistry 2007;46(19):7827-39.
2007: Connie C Lu; Eckhard Bill; Thomas Weyhermüller; Eberhard Bothe; Karl Wieghardt
The monoanionic pi-radical redox state of alpha-iminoketones in bis(ligand)metal complexes of nickel and cobalt.
Inorganic chemistry 2007;46(19):7880-9.
2007: Ruta R Kapre; Eberhard Bothe; Thomas Weyhermüller; Serena DeBeer George; Karl Wieghardt
Electronic structure of neutral and monoanionic tris(benzene-1,2-dithiolato)metal complexes of molybdenum and tungsten.
Inorganic chemistry 2007;46(14):5642-50.
2007: Edward J Reijerse; Monika Sommerhalter; Petra Hellwig; Armin Quentmeier; Dagmar Rother; Christoph Laurich; Eberhard Bothe; Wolfgang Lubitz; Cornelius G Friedrich
The unusal redox centers of SoxXA, a novel c-type heme-enzyme essential for chemotrophic sulfur-oxidation of Paracoccus pantotrophus.
Biochemistry 2007;46(26):7804-10.
2007: József Sándor Pap; Flávio Luiz Benedito; Eberhard Bothe; Eckhard Bill; Serena DeBeer George; Thomas Weyhermüller; Karl Wieghardt
Dimerization processes of square planar [PtII(tbpy)(dithiolato*)]+ radicals.
Inorganic chemistry 2007;46(10):4187-96.
2007: Yu-Fei Song; John F Berry; Eckhard Bill; Eberhard Bothe; Thomas Weyhermüller; Karl Wieghardt
Iron complexes of new pentadentate ligands containing the 1,4,7-triazacyclononane-1,4-diacetate motif. spectroscopic, electro-, and photochemical studies.
Inorganic chemistry 2007;46(6):2208-19.
2007: John F Berry; Eckhard Bill; Eberhard Bothe; F Albert Cotton; Naresh S Dalal; Sergey A Ibragimov; Narpinder Kaur; Chun Y Liu; Carlos A Murillo; Saritha Nellutla; J Micah North; Dino Villagran
A fractional bond order of 1/2 in Pd(2)(5+)--formamidinate species; the value of very high-field EPR spectra.
Journal of the American Chemical Society 2007;129(5):1393-401.
2007: Prasanta Ghosh; Keira Stobie; Eckhard Bill; Eberhard Bothe; Thomas Weyhermüller; Michael D Ward; Jon A McCleverty; Karl Wieghardt
Electronic structure of nitric oxide adducts of bis(diaryl-1,2-dithiolene)iron compounds: four-membered electron-transfer series [Fe(NO)(L)2]z (z = 1+, 0, 1-, 2-).
Inorganic chemistry 2007;46(2):522-32.
2006: John F Berry; Eckhard Bill; Eberhard Bothe; Frank Neese; Karl Wieghardt
Octahedral non-heme oxo and non-oxo Fe(IV) complexes: an experimental/theoretical comparison.
Journal of the American Chemical Society 2006;128(41):13515-28.
2006: Apurba K Patra; Eckhard Bill; Eberhard Bothe; Krzysztof Chlopek; Frank Neese; Thomas Weyhermüller; Keira Stobie; Michael D Ward; Jon A McCleverty; Karl Wieghardt
Electronic structure of mononuclear bis(1,2-diaryl-1,2-ethylenedithiolato)iron complexes containing a fifth cyanide or phosphite ligand: a combined experimental and computational study.
Inorganic chemistry 2006;45(19):7877-90.
2006: Caroline Fichtner; Christoph Laurich; Eberhard Bothe; Wolfgang Lubitz
Spectroelectrochemical characterization of the [NiFe] hydrogenase of Desulfovibrio vulgaris Miyazaki F.
Biochemistry 2006;45(32):9706-16.
2006: Krzysztof Chłopek; Eberhard Bothe; Frank Neese; Thomas Weyhermüller; Karl Wieghardt
Molecular and electronic structures of tetrahedral complexes of nickel and cobalt containing N,N'-disubstituted, bulky o-diiminobenzosemiquinonate(1-) pi-radical ligands.
Inorganic chemistry 2006;45(16):6298-307.
2006: John F Berry; Eckhard Bill; Eberhard Bothe; Serena DeBeer George; Bernd Mienert; Frank Neese; Karl Wieghardt
An octahedral coordination complex of iron(VI).
Science (New York, N.Y.) 2006;312(5782):1937-41.
2006: John F Berry; Eberhard Bothe; F Albert Cotton; Sergey A Ibragimov; Carlos A Murillo; Dino Villagran; Xiaoping Wang
Metal-metal bonding in mixed valence Ni2(5+) complexes and spectroscopic evidence for a Ni2(6+) species.
Inorganic chemistry 2006;45(11):4396-406.
2005: John F Berry; Eckhard Bill; Eberhard Bothe; Thomas Weyhermüller; Karl Wieghardt
Octahedral non-heme non-oxo Fe(IV) species stabilized by a redox-innocent N-methylated cyclam-acetate ligand.
Journal of the American Chemical Society 2005;127(33):11550-1.
2005: Laurent Benisvy; Robert Bittl; Eberhard Bothe; C David Garner; Jonathan McMaster; Stephanie Ross; Christian Teutloff; Frank Neese
Phenoxyl radicals hydrogen-bonded to imidazolium: analogues of tyrosyl D. of photosystem II: high-field EPR and DFT studies.
Angewandte Chemie (International ed. in English) 2005;44(33):5314-7.
2005: Swarnalatha Kokatam; Thomas Weyhermüller; Eberhard Bothe; Phalguni Chaudhuri; Karl Wieghardt
Structural characterization of four members of the electron-transfer series [PdII(L)2)2]n (L = o-Iminophenolate derivative; n = 2-, 1-, 0, 1+, 2+). ligand mixed valency in the monocation and monoanion with S = (1)/(2) ground states.
Inorganic chemistry 2005;44(10):3709-17.
2005: Sebastien Blanchard; Frank Neese; Eberhard Bothe; Eckhard Bill; Thomas Weyhermüller; Karl Wieghardt
Square planar vs tetrahedral coordination in diamagnetic complexes of nickel(II) containing two bidentate pi-radical monoanions.
Inorganic chemistry 2005;44(10):3636-56.
2005: Dana S Marlin; Eckhard Bill; Thomas Weyhermüller; Eberhard Bothe; Karl Wieghardt
Magnetic interactions in dinuclear Mn(III)Mn(IV) complexes covalently tethered to organic radicals: spectroscopic models for the S(2)Y(z)(*) state of photosystem II.
Journal of the American Chemical Society 2005;127(16):6095-108.
2004: Eckhard Bill; Eberhard Bothe; Phalguni Chaudhuri; Krzysztof Chlopek; Diran Herebian; Swarnalatha Kokatam; Kallol Ray; Thomas Weyhermüller; Frank Neese; Karl Wieghardt
Molecular and electronic structure of four- and five-coordinate cobalt complexes containing two o-phenylenediamine- or two o-aminophenol-type ligands at various oxidation levels: an experimental, density functional, and correlated ab initio study.
Chemistry (Weinheim an der Bergstrasse, Germany) 2004;11(1):204-24.
2004: Soumen Mukherjee; Thomas Weyhermüller; Eberhard Bothe; Karl Wieghardt; Phalguni Chaudhuri
Dinuclear and mononuclear manganese(IV)-radical complexes and their catalytic catecholase activity.
Dalton transactions (Cambridge, England : 2003) 2004;(22):3842-53.
2004: Tapan K Paine; Thomas Weyhermüller; Leonardo D Slep; Frank Neese; Eckhard Bill; Eberhard Bothe; Karl Wieghardt; Phalguni Chaudhuri
Nonoxovanadium(IV) and oxovanadium(V) complexes with mixed O, X, O-donor ligands (X = S, Se, P, or PO).
Inorganic chemistry 2004;43(23):7324-38.
2004: Kil Sik Min; Thomas Weyhermüller; Eberhard Bothe; Karl Wieghardt
Tetradentate bis(o-iminobenzosemiquinonate(1-)) pi radical ligands and their o-aminophenolate(1-) derivatives in complexes of nickel(II), palladium(II), and copper(II).
Inorganic chemistry 2004;43(9):2922-31.
2004: Ricardo García Serres; Craig A Grapperhaus; Eberhard Bothe; Eckhard Bill; Thomas Weyhermüller; Frank Neese; Karl Wieghardt
Structural, spectroscopic, and computational study of an octahedral, non-heme [Fe-NO](6-8) Series: [Fe(NO)(cyclam-ac)]2+/+/0.
Journal of the American Chemical Society 2004;126(16):5138-53.
2003: Leonardo D Slep; Ana Mijovilovich; Wolfram Meyer-Klaucke; Thomas Weyhermüller; Eckhard Bill; Eberhard Bothe; Frank Neese; Karl Wieghardt
Mixed-valent [FeIV(mu-O)(mu-carboxylato)2FeIII]3+ core.
Journal of the American Chemical Society 2003;125(50):15554-70.
2003: Diran Herebian; Eberhard Bothe; Frank Neese; Thomas Weyhermüller; Karl Wieghardt
Molecular and electronic structures of bis-(o-diiminobenzosemiquinonato)metal(II) complexes (Ni, Pd, Pt), their monocations and -anions, and of dimeric dications containing weak metal-metal bonds.
Journal of the American Chemical Society 2003;125(30):9116-28.
2003: Prasanta Ghosh; Ameerunisha Begum; Diran Herebian; Eberhard Bothe; Knut Hildenbrand; Thomas Weyhermüller; Karl Wieghardt
Coordinated o-dithio- and o-iminothiobenzosemiquinonate(1-) pi radicals in [MII(bpy)(L*)](PF6) complexes.
Angewandte Chemie (International ed. in English) 2003;42(5):563-7.
2002: Hyungphil Chun; Eckhard Bill; Eberhard Bothe; Thomas Weyhermüller; Karl Wieghardt
Octahedral (cis-cyclam)iron(III) complexes with O,N-coordinated o-iminosemiquinonate(1-) pi radicals and o-imidophenolate(2-) anions.
Inorganic chemistry 2002;41(20):5091-9.
2002: Xianru Sun; Hyungphil Chun; Knut Hildenbrand; Eberhard Bothe; Thomas Weyhermüller; Frank Neese; Karl Wieghardt
o-Iminobenzosemiquinonato(1-) and o-amidophenolato(2-) complexes of palladium(II) and platinum(II): a combined experimental and density functional theoretical study.
Inorganic chemistry 2002;41(16):4295-303.
2001: Diran Herebian; Eberhard Bothe; Eckhard Bill; Thomas Weyhermüller; Karl Wieghardt
Experimental evidence for the noninnocence of o-aminothiophenolates: coordination chemistry of o-iminothionebenzosemiquinonate(1-) pi-radicals with Ni(II), Pd(II), Pt(II).
Journal of the American Chemical Society 2001;123(41):10012-23.
2001: Hyungphil Chun; Claudio N Verani; Phalguni Chaudhuri; Eberhard Bothe; Eckhard Bill; Thomas Weyhermüller; Karl Wieghardt
Molecular and electronic structure of octahedral o-aminophenolato and o-iminobenzosemiquinonato complexes of V(V), Cr(III), Fe(III), and Co(III). Experimental determination of oxidation levels of ligands and metal ions.
Inorganic chemistry 2001;40(17):4157-66.
2001: P Chaudhuri; Claudio N Verani; E Bill; Eberhard Bothe; Thomas Weyhermüller; Karl Wieghardt
Electronic structure of bis(o-iminobenzosemiquinonato)metal complexes (Cu, Ni, Pd). The art of establishing physical oxidation states in transition-metal complexes containing radical ligands.
Journal of the American Chemical Society 2001;123(10):2213-23.
2000: P Ulanski; Eberhard Bothe; Knut Hildenbrand; Clemens von Sonntag
Free-radical-induced chain breakage and depolymerization of poly(methacrylic acid): equilibrium polymerization in aqueous solution at room temperature.
Chemistry (Weinheim an der Bergstrasse, Germany) 2000;6(21):3922-34.
2000: A Adhikary; Eberhard Bothe; V Jain; Clemens von Sonntag
Pulse radiolysis of the DNA-binding bisbenzimidazole derivatives Hoechst 33258 and 33342 in aqueous solutions.
International journal of radiation biology 2000;76(9):1157-66.
2000: Bas de Bruin; E Bill; Eberhard Bothe; T Weyhermüller; Karl Wieghardt
Molecular and electronic structures of bis(pyridine-2,6-diimine)metal complexes [ML2](PF6)n (n = 0, 1, 2, 3; M = Mn, Fe, Co, Ni, Cu, Zn).
Inorganic chemistry 2000;39(13):2936-47.